我室侯旭教授在 nanotoday 上发表论文：Tannic acid modified single nanopore with multivalent metal ions recognition and ultra-trace level detection文章链接：https://www.sciencedirect.com/science/article/pii/S1748013220300372摘要：Artificial single nanopore as a promising tool for chemical and biological studies, such as ionic detection, DNA sequencing, molecular sensing/separation, nanofluidics a...

我室李剑锋教授在 Science Advances 上发表论文：Real-time detection of single-molecule reaction by plasmon-enhanced spectroscopy文章链接：https://advances.sciencemag.org/content/6/24/eaba6012摘要：Determining structural transformations of single molecules (SMs) is an important fundamental scientific endeavor. Optical spectroscopies are the dominant tools used to unravel the physical and chemical ...

我室洪文晶教授在 Science Advances 上发表论文：Cross-plane transport in a single-molecule two-dimensional van der Waals heterojunction文章链接：https://advances.sciencemag.org/content/6/22/eaba6714摘要：Two-dimensional van der Waals heterojunctions (2D-vdWHs) stacked from atomically thick 2D materials are predicted to be a diverse class of electronic materials with unique electronic properties. ...

我室龙腊生教授在 ACIE 上发表论文：The Mechanism of the Magnetodielectric Response in a Molecule‐Based Trinuclear Iron Cluster Material文章链接：https://onlinelibrary.wiley.com/doi/10.1002/anie.202007813摘要：Magnetodielectric response mechanisms are critical for the rational design and synthesis of molecule‐based magnetodielectric materials. Herein, the magnetodielectric response was investig...

我室任斌教授课题组运用自主研发的等离激元传感器，分离界面折射率中的体相折射率和表面折射率贡献，定量描述和测量了界面折射率。相关研究成果以“Determining the Interfacial Refractive Index via Ultrasensitive Plasmonic Sensors”为题发表于美国化学会志（J. Am. Chem. Soc., DOI:10.1021/jacs.0c01907）。折射率是反映光与介质相互作用的重要物理量。基于表面等离激元对周围环境折射率变化的敏感响应，等离激元传感器...

我室苏培峰教授在 J. Phys. Chem. Lett. 上发表论文：A Novel Valence-Bond-Based Automatic Diabatization Method by Compression文章链接：https://pubs.acs.org/doi/10.1021/acs.jpclett.0c01466摘要：A novel valence-bond-based automatic diabatization method by compression, called valence-bond-based compression approach for dibatization (VBCAD), is presented in this Letter. It is a “black-box” type met...

我室李剑锋教授在 J. Am. Chem. Soc. 上发表论文：Probing Electric Field Distributions in the Double Layer of a Single-Crystal Electrode with Angstrom Spatial Resolution using Raman Spectroscopy文章链接：https://pubs.acs.org/doi/10.1021/jacs.0c05162摘要：The electrical double layer (EDL) is the extremely important interfacial region involved in many electrochemical reactions, and it is the subject...

我室徐海超教授课题组在有机光电合成研究方面取得新进展，相关成果以“Scalable Photoelectrochemical Dehydrogenative Cross-Coupling of Heteroarenes with Aliphatic C–H Bonds”为题在线发表于《德国应用化学》 (Angew. Chem. Int. Ed., DOI: 10.1002/anie.202005724)。C–H/C–H脱氢偶联具有较高的步骤和原子经济性，且使用易得的原料，其是构筑C–C键的最有效方法之一。 另一方面，杂芳烃是药物、天然产物和功能材料中的...

我室徐海超课题组与程俊课题组合作，在有机电合成研究方面取得新进展，相关成果以“Site-selective electrooxidation of methylarenes to aromatic acetals”为题在线发表于《自然·通讯》(Nat. Commun. 2020, 11, 2706)。  醛可参与多种反应，是用途最为广泛的有机合成中间体之一。其中芳香醛已被用于合成精细化学品、营养食品、功能材料和药物等。由于甲基芳烃稳定、易得，且易于处理，其苄位氧化是制备芳香醛的一种很有吸引力...

近日，我室王斌举教授课题组与伊利诺伊大学赵惠民教授课题组合作，报道了光诱导的酶催化反应用于分子间碳碳交叉偶联反应，相关研究成果以“Photoenzymatic enantioselective intermolecular radical hydroalkylation”为题在线发表于Nature。相比于传统化学合成，基于酶催化的生物合成具有反应条件温和、选择性高以及绿色可持续等优势，一直是一个重要的研究领域。然而，酶催化反应类型往往局限于酶本身专一催化的反应，这极大...